arXiv:2605.00678v1 Announce Type: new Abstract: Aerosol Optical Depth (AOD) retrieval is essential for Earth observation, supporting applications from air quality monitoring to climate studies. Conventional physics-based AOD retrieval methods formulate the problem as a pixel-wise inversion, relying on radiative transfer modeling, memory-intensive look-up tables, and auxiliary meteorological data. While recent data-driven approaches have shown promise, many fail to exploit the spatial-spectral coherence of hyperspectral imagery, leading to spatially inconsistent and noise-sensitive retrievals. We present the first study exploring Foundation AI models for AOD retrieval and propose ViTCG, a Vision Transformer with Channel-wise Grouping-based spatial regression framework that reduces retrieval bias and error. ViTCG uses hyperspectral top-of-atmosphere radiance as input and jointly models spatial context and spectral information. Validation with PACE radiance observations demonstrates a 62% reduction in mean squared error compared to state-of-the-art foundation models, including Prithvi, and produces spatially coherent AOD fields.